Using everyone else's hard work
, soupdragon and ChristmasQuizzer theories kind of work:
WHI CHF ILM Reign of Fire, Shaft, Vice
Christian Bale
THA TST ARS Fandango, Man of Steel, Code Breaker
Kevin Costner
TWO OFT HEA Cocktail, Magnolia , Valkarie
Tom Cruise
CTO RSL IST Interstella (?) The Martian, Rounders
Matt Damon
EDC AME OUT Airforce One, (?), Patriot Games
Harrison Ford
INN INE TEE ? , Maverick , Nell
Jodie Foster
NNI NET YTH Salt, Ted 2, Seven - can't find a connection
REE AND WHI ?, Fracture, ?
CHO THE RFI ?, Lucy, ?
LMS TAR RIN Alexander, Mr & Mrs Smith, ?
Angelina Jolie
GAN OTH ERA ?, Capone, Gladiator can't find connection
CTO RLI STE Fury, Moneyball, Troy
Brad Pitt
DCA MEO UTT The Chase, Sneakers, The Sting
Robert Redford
HES AME YEA Hook, Michael Collins , Notting hill
Julia Roberts
RTH EYA REB Bright, Focus, ?
Will Smith
ASE DON THE Flight, Twister, can't find connection
NOV ELS BYT Philidelphia, The Bee Movie, Split no connection
HES AME AUT HOR Twelve Monkeys (?), Blackbird, Jude, Quills
Kate Winslet
The "?" are either the film is wrong or I have split the letters wrong
So, using the actors listed, The Firm (Tom Cruise) and The Pelican Brief (Julia Roberts) somewhat fits.
I could, however, be completely wrong 