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You would need to contact your old employer as per the FAQ:
Whether vouchers in a Childcare Voucher account may be returned to you will depend on the details of your Salary Sacrifice agreement and employment contract with the employer who made the deductions.
Please note that it is often the case that the Salary Sacrifice agreement does not allow for the reversal of Childcare Vouchers back to salary.
Edenred cannot arrange a cash alternative to any surplus Childcare Vouchers under any circumstances – this is because Edenred play no part in salary deductions.
Your employer placed the instruction to create an account and deposit the vouchers on your behalf and the Salary Sacrifice agreement will determine the rules of the scheme. This agreement still applies even if you are no longer with the same employer.
Childcare Vouchers have no expiry date and can be used for registered/approved care until the September following your youngest child's fifteenth birthday, or sixteenth if they have a disability. Types of care available can include breakfast clubs, after school care, holiday clubs, and in some cases, tuition.
Please refer to your Salary Sacrifice agreement in the first instance if you have any further queries. If you do not hold a copy of this, the HR/Payroll team may be able to assist you.