I appreciate that this thread is now 5 years out of date, but I've just come across it by accident & thought I'd post my experience for anybody else reading who has the same problem.
The OPs' problem could've been written by me, 11 years ago. My DH immediately got very angry, every time our newborn daughter cried. I spent the first year of her life, at least, trying to make sure my baby didn't cry, in an effort to keep the peace.
It turned out that the birth of our daughter had triggered PTSD in my husband, who had been physically and emotionally abused by both his parents, and sexually abused by his mother. This had been so 'normalised' to him that neither of us had even been aware that his childhood had been anything but normal. (he was 23 when our daughter was born).
The birth also triggered abandonment issues for him, in that after being abused and abandoned as a child, I was now 'abandoning' him as our daughter needed to come first. This was made worse by the fact that his mother had spent her life telling him she never wanted a son, but a daughter instead (and our child, his 'replacement', was a girl!).
11 years later, and after a LOT of effort from him (and me), he is now much, much better - and we have other children now, too. I'm not sure the choice I made was the smart one (like other posters, due to my DH losing his temper there was a time when it wasn't safe to leave the baby with him) - but I chose to believe in him, and he did put the effort in & get better - and we both adore our family now.
What I'm saying is, maybe it's just normal 'feeling out of control' symptoms - or maybe it's something more serious. If somebody had told me 10 years ago what I know now about DH & his family, there's no way I'd have believed them. Maybe it isn't just your DH needing to grow up / acting out.
Saying that though, if there is a more serious problem, you won't fix it on your own - it will take a serious amount of commitment from your DH, and huge amount of support & tolerance from you too. Choosing to stay & work through it is not the easy option.